AVS 66th International Symposium & Exhibition
    2D Materials Wednesday Sessions
       Session 2D+AS+MI+NS-WeM

Invited Paper 2D+AS+MI+NS-WeM3
Interfacial and Topological Superconductivity in 2D Layers Studied by Spin-Resolved Scanning Tunneling Spectroscopy

Wednesday, October 23, 2019, 8:40 am, Room A216

Session: 2D Materials Characterization by Scanning Probe Microscopy and Spectroscopy
Presenter: Roland Wiesendanger, University of Hamburg, Germany
Correspondent: Click to Email

In this presentation, we will first focus on interfacial superconductivity in novel types of heterostructures. In particular, we will present a low-temperature SP-STS study of ultrathin FeTe1-xSex (x = 0, 0.5) films grown on prototypical Bi-based bulk topological insulators. We observe fully developed U-shaped superconducting gaps in FeTe0.5Se0.5 layers of one unit cell (UC) thickness with a transition temperature (Tc) of ~11 K, close to the one of the corresponding bulk system (Tc ~ 14.5 K) [1]. Surprisingly, we also find clear evidence for superconductivity up to Tc ~ 6 K for one UC thick FeTe layers grown on Bi2Te3 substrates [2], in contrast to the non-superconducting FeTe bulk compound which exhibits bicollinear antiferromagnetic (AFM) order in a wide temperature range up to 70 K. Even more surprisingly, detailed investigations of the atomic-scale spin-resolved local density of states by SP-STS reveal that superconductivity in one UC layers of FeTe grown on Bi2Te3 appears to spatially coexist with bi-collinear AFM order. By using 3D-vector-resolved SP-STM techniques [3] we find an unusual reorientation of the diagonal double-stripe spin structure at Fe1+yTe thin film surfaces [4]. Moreover, variable-temperature SP-STM studies [5] reveal an enhanced Néel temperature for AFM spin ordering of the ultrathin FeTe films grown on topological insulators [6]. These findings open novel perspectives for theoretical studies of competing orders in Fe-based superconductors as well as for experimental investigations of exotic phases in heterostructures of topological insulators and superconducting layers.

In a second part, we will address experimental and theoretical studies of monolayer topological superconductivity and chiral Majorana edge modes in model-type 2D magnetic Fe islands on elemental superconducting Re [7]. In particular, we demonstrate that interface engineering by an atomically thin oxide layer is crucial for driving the studied hybrid system into a topologically non-trivial state as confirmed by theoretical calculations of the topological invariant, the Chern number.

This work is supported by the EU via the ERC Advanced Grant No. 786020 “ADMIRE”.

[1] A. Kamlapure et al., Phys. Rev. B 95, 104509 (2017).

[2] S. Manna et al., Nature Commun. 8, 14074 (2017).

[3] S. Meckler et al., Rev. Sci. Instrum. 80, 023708 (2009).

[4] T. Hänke et al., Nature Commun. 8, 13939 (2017).

[5] J. Warmuth et al., NPG Quantum Materials 3, 21 (2018).

[6] U. R. Singh et al., Phys. Rev. B 97, 144513 (2018).

[7] A. Palacio-Morales, E. Mascot, S. Cocklin, H. Kim, S. Rachel, D. K. Morr, and R. Wiesendanger, arXiv:1809.04503 (2018).