AVS 63rd International Symposium & Exhibition
    Magnetic Interfaces and Nanostructures Monday Sessions
       Session MI+2D+AC-MoM

Paper MI+2D+AC-MoM4
Microscopic Magnetic Structures in Dy/Y Superlattices Measured by Polarized Neutron Reflectometry with Off-specular Scattering

Monday, November 7, 2016, 9:20 am, Room 101C

Session: Chiral Magnetism (8:20-10:20 am)/Magnetism and Spin Orbit Effects at Interfaces and Surfaces: Recent Experimental and Theoretical Advances (10:40 am - 12:00 pm)
Presenter: Gary Mankey, University of Alabama
Authors: G. Mankey, University of Alabama
J. Yu, University of Alabama
P. LeClair, University of Alabama
R. Fishman, Oak Ridge National Laboratory
J.L. Robertson, Oak Ridge National Laboratory
H. Ambaye, Oak Ridge National Laboratory
V. Lauter, Oak Ridge National Laboratory
H. Lauter, Oak Ridge National Laboratory
Correspondent: Click to Email

Epitaxial Dy/Y superlattices with vertically-oriented c-axes, nanometer-scale layer thicknesses and 8-80 repeats were fabricated by magnetron sputtering on a-sapphire substrates with Nb buffer layers. The samples are designed to study how helical magnetic structures in Dy are modified by coupling through non-magnetic Y layers. X-ray characterization was used to evaluate the crystallographic orientations and interface widths of the superlattices. The macroscopic magnetic properties were characterized by low-temperature magnetometery that shows cooling in a 1 T in-plane field results in significant ferromagnetically-aligned moments below magnetic transition temperatures of approximately 150 K. The microscopic magnetic structures were investigated by polarized neutron reflectometry with off-specular scattering (PNROS) with variable magnetic fields in a temperature range from 300K down to 5K. PNROS confirms the magnetic transition and shows how the microscopic magnetic structures of the multilayered samples change with temperature. The ordering of the helical modulation is sensitive to the interfacial roughness of the multilayers as well as the magnetic and temperature history of the samples. The turn angles of the helical magnetic moment can be extracted from fitting the data. When the samples are cooled from room temperature to 5 K in a 10 mT in-plane applied magnetic field, the helical magnetic structures appear to decompose into lateral domains of opposite chirality, as evidenced by strong off-specular Bragg sheets. The Bragg sheets originate from the magnetic peaks associated with the helical magnetic ordering. The strength of the scattering from these sheets varies from sample to sample, suggesting that some samples may have a preferred chirality, due to differences in the microscopic film structure.

The authors gratefully acknowledge financial support from DOE award DE-FG02-08ER46499. A portion of this research used resources at the Spallation Neutron Source, a DOE Office of Science User Facility operated by the Oak Ridge National Laboratory.