Pacific Rim Symposium on Surfaces, Coatings and Interfaces (PacSurf 2016)
    Nanomaterials Tuesday Sessions
       Session NM-TuE

Paper NM-TuE5
Structural and Electrical Properties of Electromigrated Au Nanogaps

Tuesday, December 13, 2016, 7:00 pm, Room Hau

Session: Nanofabrication and Nanodevices II
Presenter: Tomoyuki Ito, Tokyo University of Agriculture & Technology, Japan
Authors: T. Ito, Tokyo University of Agriculture & Technology, Japan
K. Inoue, Tokyo University of Agriculture & Technology, Japan
J. Shirakashi, Tokyo University of Agriculture & Technology, Japan
Correspondent: Click to Email

Au nanogaps have been attractive for the fabrication of single-molecule devices. For this reason, many different approaches of Au nanogaps have been reported, including electromigration [1], break junction [2] and electroplating [3]. We have already reported on fabricating narrower Ni nanogaps by controlling tunnel resistance of the nanogaps using field-emission-induced electromigration. We call this method “activation” [4, 5]. In this report, the application of activation to Au nanogaps is investigated in comparison with that of Ni nanogaps.

Under room temperature and vacuum condition, the activation was applied to initial Au nanogaps with a separation of around 50 nm. The initial Au nanogaps showed high tunnel resistance of more than 500 TΩ. After performing the activation with the preset current Is of above 300 nA, the tunnel resistance of Au nanogaps gradually decreased to less than 10 MΩ. Activation properties of Au nanogaps are quite similar to those of Ni nanogaps ever reported [4, 5]. Thus, the results imply that the tunnel resistance of Au nanogaps can be controlled in the same way as that of Ni nanogaps using activation.

References

[1] K. Yoshida, K. Shibata, and K. Hirakawa, Phys. Rev. Lett. 115 (2015) 138302.

[2] J. M. van Ruitenbeek, A. Alvarez, I. Pineyro, C. Grahmann, P.Joyez, M. H. Devoret, D. Esteve, and C. Urbina, Rev. Sci. Instrum. 67 (1995) 108-111.

[3] B. Liu, J. Xiang, J. H. Tian, C. Zhong, B. W. Mao, F. Z. Yang, Z. B. Chen, S. T. Wu, and Z. Q. Tian, Electrochim. Acta. 50 (2005) 3041-3047.

[4] S. Kayashima, K. Takahashi, M. Motoyama, and J. Shirakashi, Jpn. J. Appl. Phys. 46 (2007) L907-L909.

[5] W. Kume, Y. Tomoda, M. Hanada, and J. Shirakashi, J Nanosci. Nanotechnol. 10 (2010) 7239-7243.