AVS 64th International Symposium & Exhibition
    Nanometer-scale Science and Technology Division Tuesday Sessions
       Session NS+EM+MI+SS-TuM

Invited Paper NS+EM+MI+SS-TuM12
The Exciting Physics of Spin Chains Coupled to a Metallic Substrate

Tuesday, October 31, 2017, 11:40 am, Room 19

Session: Nanoscale Electronics and Magnetism
Presenter: Roland Wiesendanger, University of Hamburg, Germany
Correspondent: Click to Email

A magnetic nanowire on the surface of a spin-orbit coupled s-wave superconductor is a fascinating platform, which has been proposed for observing the emergence of zero-energy Majorana bound states at the ends of the wires [1]. Majorana fermions can encode topological qubits and ultimately provide a new direction in topological quantum computation [2]. Most recently, evidences for topologically non-trivial end-states were experimentally found for self-assembled ferromagnetic Fe nanowires on superconducting Pb(110) substrates by using scanning tunneling microscopy and spectroscopy (STM/S) as well as non-contact atomic force microscopy methods [3-6]. However, self-assembled nanowires of Fe on Pb surfaces have unavoidable limitations, such as (1) intermixing of atomic species of the nanowire and the substrate during the annealing process, and (2) uncontrolled length and orientation of the nanowires.

Here, we demonstrate the fully-controlled bottom-up fabrication of artificial 1D atomic chains from individual magnetic Fe adatoms on high spin-orbit coupled non-superconducting Pt(111) and superconducting Re(0001) substrates by utilizing STM-based atom-manipulation techniques at T=350 mK. Spin-polarized STM measurements indicate the presence of non-collinear spin textures, i.e. spin spiral ground states, stabilized by interfacial Dzyaloshinskii-Moriya interactions similar to self-assembled Fe chains on Ir(001) investigated earlier [7]. The problem of intermixing is avoided by the low-temperature fabrication of the chain and an appropriate choice of the substrate, while single-atom manipulation allows the construction of chains with a given number of atoms and orientation. Tunneling spectra measured spatially resolved on the Fe-atom chain on Re(0001) reveal the evolution of the local density of states (LDOS) inside the superconducting gap as well as the development of zero-energy bound states at the ends of the chain, which are distinguishable from trivial end states by systematically increasing the number of atoms within the Fe-atom chain. The experimental results will be compared with model-type calculations supporting the interpretation of the spectroscopic signatures at the ends of the chains as Majorana bound states.

(work done together with Howon Kim and Khai Ton That).

References

[1] H.-Y. Hui et al., Sci. Rep.. 5, 8880 (2015).

[2] J. Alicea et al., Nature Phys. 7, 412 (2011).

[3] S. Nadj-Perge et al., Science 346, 602 (2014).

[4] M. Ruby et al., Phys. Rev. Lett. 115, 197204 (2015).

[5] R. Pawlak et al., NPJ Quantum Information 2, 16035 (2016).

[6] B. E. Feldman et al., Nature Phys. 13, 286 (2017).

[7] M. Menzel et al., Phys. Rev. Lett. 108, 197204 (2012).