AVS 55th International Symposium & Exhibition | |
Surface Science | Thursday Sessions |
Session SS1+NC-ThA |
Session: | Water-Surface Interactions |
Presenter: | B.D. Kay, Pacific Northwest National Laboratory |
Authors: | B.D. Kay, Pacific Northwest National Laboratory J.L. Daschbach, Pacific Northwest National Laboratory Z. Dohnálek, Pacific Northwest National Laboratory G.A. Kimmel, Pacific Northwest National Laboratory J. Matthiesen, Pacific Northwest National Laboratory N.G. Petrik, Pacific Northwest National Laboratory R.S. Smith, Pacific Northwest National Laboratory T. Zubkov, Pacific Northwest National Laboratory |
Correspondent: | Click to Email |
Molecular beam scattering, programmed desorption (both TPD and isothermal), and vibrational spectroscopy are used to study the chemical kinetics and reaction dynamics of molecular processes occurring both on the surface and within the bulk of amorphous and crystalline ice films. Molecular beams are used to synthesize chemically and structurally tailored thin films on various substrates including Pt(111), Pd(111), C(111) and FeO(111). These films can have morphologies ranging from dense and smooth, to highly porous depending on growth conditions. The precise control of the film structure allows physiochemical processes such as densification, crystallization, diffusion, isotope exchange, solvation, and dewetting to be studied in detail. The experimental methods, results, and their relevance to supercooled water, astrophysical icy bodies, wetting phenomena and nanoporous materials will be presented. Pacific Northwest National Laboratory is a multiprogram national laboratory operated for the U.S. Department of Energy by Battelle Memorial Institute under contract DE-AC06-76RLO 1830.