AVS 54th International Symposium
    Surface Science Monday Sessions
       Session SS2-MoM

Paper SS2-MoM8
Novel Superstructure of Thin Pb Film on Si(111) Induced by the Interplay of Quantum Well States and Interfacial Adsorbates

Monday, October 15, 2007, 10:20 am, Room 611

Session: Surface Structure, Growth, and Etching of Silicon and Germanium
Presenter: A.A. Khajetoorians, The University of Texas at Austin
Authors: A.A. Khajetoorians, The University of Texas at Austin
H. Eisele, The University of Texas at Austin
S.Y. Qin, The University of Texas at Austin
C.-K. Shih, The University of Texas at Austin
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Epitaxial thin Pb films on Si(111) are well known to exhibit pronounced QSE manifested by the phase matching of the Fermi wavelength and the layer thickness, giving rise to bilayer oscillation as well as a re-entrant quantum beats of longer periodicity. Such quantum oscillation phenomena have been observed in preferred film thickness, the location of quantum well states, as well as superconductivity. This work reveals yet another intriguing phenomenon manifested by the QSE: Formation of a novel superstructure resulting from the interplay of the quantum well state of the metal film and the cesium adsorbates at the interface of Si(111) substrate and Pb thin film overlayers. The superstructure consists of a periodicity of about 8 nm, incommensurate with the Si(111) 7x7 periodicity. Moreover, there is a dependence of the actual periodicity and orientation on the film thickness. This work is supported is supported by: IGERT-NSF: DGE-054917; FRG: (DMR-0306239, DMR-0606485), Alexander von Humboldt Foundation.